Investigation of LSPR and Raman Sensing Sensitivities of Circular Metal-insulator-metal (MIM) Cavity Arrays

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dc.contributor.advisor Lienau, Christoph (Prof. Dr.)
dc.contributor.author Dai, Fang
dc.date.accessioned 2019-08-30T11:39:20Z
dc.date.available 2019-08-30T11:39:20Z
dc.date.issued 2021-07-03
dc.identifier.uri http://hdl.handle.net/10900/92172
dc.identifier.uri http://nbn-resolving.de/urn:nbn:de:bsz:21-dspace-921720 de_DE
dc.identifier.uri http://dx.doi.org/10.15496/publikation-33553
dc.description.abstract We investigate the performance of vertical metal-insulator-metal (MIM) structures as refractive index (RI) sensors and surface enhanced Raman scattering (SERS) substrates. The disc-on-film structures with different geometrical parameters and different spacer configurations were studied systematically by experiments and simulations. The circular Fabry-Pérot (FP) cavity model was applied to describe the cavity plasmon modes, which were divided into edge cavity modes and surface cavity modes, showing different optical response to wet etching, RI sensing and SERS. The dependencies of cavity plasmon modes as a function of periodicity, cavity radius and cavity height were studied. The reasons for different line shapes of far-field spectra were revealed. The influences of varying spacers on the locations of 'hot spots' and resonance wavelengths were systematically studied. The 'hot spots' of cavity plasmon modes were exposed by wet etching. The RI sensitivities of MIM structures were thoroughly studied including different types of plasmonic modes, sensing based on spectral shifts and intensity changes, and bulk/molecular RI sensing configurations. Notable SERS enhancement factors (EFs) were achieved by underetching. EF peaks attributed to different orders of cavity plasmon modes were observed in both experiments and simulations. Good qualitative agreement was found between the experimental and simulated results. A similar dependency of the effective SERS EF as a function of cavity radius was found for vertical disc dimers compared to disc-on-film substrates. en
dc.language.iso en de_DE
dc.publisher Universität Tübingen de_DE
dc.rights ubt-podok de_DE
dc.rights.uri http://tobias-lib.uni-tuebingen.de/doku/lic_mit_pod.php?la=de de_DE
dc.rights.uri http://tobias-lib.uni-tuebingen.de/doku/lic_mit_pod.php?la=en en
dc.subject.classification Physik , Nanopartikel de_DE
dc.subject.ddc 500 de_DE
dc.subject.ddc 530 de_DE
dc.subject.other Plasmons en
dc.subject.other nanoparticles en
dc.subject.other optische Eigenschaften de_DE
dc.subject.other Fabry-Pérot interferometers en
dc.subject.other optical properties en
dc.subject.other oberflächenverstärkte Raman-Streuung de_DE
dc.subject.other Raman e ect en
dc.subject.other Brechungsindexsensor de_DE
dc.subject.other Fabry-Pérot-Resonator de_DE
dc.subject.other surface enhanced en
dc.subject.other Plasmonen de_DE
dc.subject.other sensing en
dc.title Investigation of LSPR and Raman Sensing Sensitivities of Circular Metal-insulator-metal (MIM) Cavity Arrays en
dc.type PhDThesis de_DE
dcterms.dateAccepted 2019-07-03
utue.publikation.fachbereich Physik de_DE
utue.publikation.fakultaet 7 Mathematisch-Naturwissenschaftliche Fakultät de_DE
utue.publikation.noppn yes de_DE

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